Detection and characterization of chemical aerosol using laser-trapping single-particle Raman spectroscopy

Aimable Kalume, Leonid A. Beresnev, Joshua Santarpia, Yong Le Pan

Research output: Contribution to journalArticle

15 Scopus citations

Abstract

Detection and characterization of the presence of chemical agent aerosols in various complex atmospheric environments is an essential defense mission. Raman spectroscopy has the ability to identify chemical molecules, but there are limited numbers of photons detectable from single airborne aerosol particles as they are flowing through a detection system. In this paper, we report on a single-particle Raman spectrometer system that can measure strong spontaneous, stimulated, and resonance Raman spectral peaks from a single laser-trapped chemical aerosol particle, such as a droplet of the VX nerve agent chemical simulant diethyl phthalate. Using this system, time-resolved Raman spectra and elastic scattered intensities were recorded to monitor the chemical properties and size variation of the trapped particle. Such a system supplies a new approach for the detection and characterization of single airborne chemical aerosol particles.

Original languageEnglish (US)
Pages (from-to)6577-6582
Number of pages6
JournalApplied optics
Volume56
Issue number23
DOIs
StatePublished - Aug 10 2017

ASJC Scopus subject areas

  • Atomic and Molecular Physics, and Optics
  • Engineering (miscellaneous)
  • Electrical and Electronic Engineering

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